01 - Preheat oven to 350°F (175°C). Line two baking sheets with parchment paper.
02 - In a medium bowl, whisk together all-purpose flour, unsweetened cocoa powder, baking soda, and salt until fully combined.
03 - In a large bowl, beat unsalted butter and granulated sugar with an electric mixer until light and fluffy. Incorporate the egg by mixing until smooth.
04 - Add buttermilk and vanilla extract to the butter mixture. Gradually incorporate the dry ingredient blend, mixing until a smooth batter forms.
05 - Using a spoon or cookie scoop, drop 24 even rounds of batter spaced 2 inches apart onto prepared baking sheets.
06 - Bake for 10 to 12 minutes or until cake surfaces are set and spring back lightly when touched. Transfer to a cooling rack and cool completely.
07 - In a clean bowl, beat softened butter until creamy. Add powdered sugar, marshmallow creme, vanilla extract, and a pinch of salt. Beat until mixture is light and fluffy.
08 - Divide filling evenly among three bowls. Leave one bowl plain, color one with red food coloring, and the third with blue food coloring, mixing until colors are vibrant.
09 - Pipe or spoon a generous layer of filling onto the flat side of half the cakes. Top with the remaining cakes to create sandwiches.
10 - Roll filled edges in patriotic sprinkles or pipe additional colored frosting on top, as desired. Chill for 30 minutes for firmer handling before serving.